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Eco-friendly catalytic systems based on MgO- Supporting carbon materials for the Friedländer condensation

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dc.contributor.authorGodino Ojer, Marina
dc.contributor.authorLópez Peinado, Antonio José
dc.contributor.authorPrzepiórski, J.
dc.contributor.authorPérez Mayoral, María Elena
dc.contributor.authorSoriano, E.
dc.contributor.authorMartín Aranda, Rosa María
dc.date.accessioned2025-01-09T12:49:59Z
dc.date.available2025-01-09T12:49:59Z
dc.date.issued2014-12
dc.descriptionEsta es la versión aceptada del artículo. La versión registrada fue publicada por primera vez en ChemCatChemVolume 6, Issue 12, Pages 3440 - 3447, está disponible en línea en el sitio web del editor: https://doi.org/10.1002/cctc.201402602. This is the accepted version of the article. The registered version was first published in ChemCatChemVolume 6, Issue 12, Pages 3440 - 3447, it is available online on the publisher's website: https://doi.org/10.1002/cctc.201402602.
dc.description.abstractCarbon-supported MgO materials are excellent and sustainable catalysts for the synthesis of N-containing heterocyclic compounds by the Friedländer condensation under mild, solvent-free conditions. The results reported herein indicate that MgO is the most active catalytic species that accelerates the reaction compared with the catalytic behavior observed for the carbon material Norit RX3. On the basis of DFT calculations, a reaction mechanism that involves dual activation of the reacting structures by the catalyst is proposed. Oxide, outside: MgO supported on carbon is able to catalyze the synthesis of interesting N-containing heterocyclic compounds efficiently under mild conditions. MgO on the carbon surface is responsible for the catalytic behavior. These carbon materials are environmentally friendly catalysts for the Friedländer reaction.en
dc.description.versionversión final
dc.identifier.citationM. Godino-Ojer, A. J. López- Peinado, R. M. Martín-Aranda, J. Przepiórski, E. Pérez-Mayoral, and E. Soriano (2014) Eco-friendly Catalytic Systems Based on MgO- Supporting Carbon Materials for the Friedländer Condensation ChemCatChemVolume 6, Issue 12, Pages 3440 - 344, https://doi.org/10.1002/cctc.201402602
dc.identifier.doihttps://doi.org/10.1002/cctc.201402602
dc.identifier.issn1867-3899 e-ISSN:1867-3880
dc.identifier.urihttps://hdl.handle.net/20.500.14468/25150
dc.journal.issue12
dc.journal.titleChemCatChem
dc.journal.volume6
dc.language.isoen
dc.page.final3447
dc.page.initial3440
dc.publisherWiley
dc.relation.centerFacultad de Ciencias
dc.relation.departmentQuímica Inorgánica y Química Técnica
dc.rightsinfo:eu-repo/semantics/openAccess
dc.rights.urihttp://creativecommons.org/licenses/by-nc-nd/4.0/deed.es
dc.subject23 Química
dc.subject.keywordscarbonen
dc.subject.keywordsmagnesiumen
dc.subject.keywordsnitrogen heterocyclesen
dc.subject.keywordsreaction mechanismsen
dc.subject.keywordssupported catalystsen
dc.titleEco-friendly catalytic systems based on MgO- Supporting carbon materials for the Friedländer condensationen
dc.typeartículoes
dc.typejournal articleen
dspace.entity.typePublication
relation.isAuthorOfPublicationa0e31477-6806-4f00-afdc-90c4136f232e
relation.isAuthorOfPublicationbafbca28-7ba9-4a29-b350-ebdcbc2381bb
relation.isAuthorOfPublication.latestForDiscoverya0e31477-6806-4f00-afdc-90c4136f232e
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